The Citi Driver's Edge card will pay 6% at gas stations for the first year (3% thereafter), but the rewards must be applied to auto maintenace, purchase, or lease.
The Chase Freedom card will net you 3.75% at gas stations if you wait to redeem your rewards in $200 increments.
The AmEx Blue Cash card goes up to 5% at gas stations, but it's tiered, so your results will depend on how much you spend.
There are other good gas cards too. To easily compare how much each will pay you for your gas station spending (and other spending if you have other spending on your card) and apply for the best card, you can use this rewards calculator:
http://www.creditcardtuneup.com/
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